WEO3: Calculated energiesa at the B3LYP/Genb Level

system Energy of D3 equilibrium geometry Relative energy,c D3h,
imaginary modes (cm-1)
Relative energy,c C2v,
imaginary modes (cm-1)
3D
Image
for each
Geometry
(GaL3)
Sc(III) -1560.73046551 [-1560.602408] 6.1 [7.7], 60i (A1") 5.6 [7.3], 45i (A2)
Ti(IV)+ -1649.21399795 [-1649.082561] 7.5 [9.5], 68i (A1") 6.1 [8.7] 48i (A2)
Co(III) -2182.66123958 [-2182.523866]e 71.1 [77.6], 40id 64.4 [60.4], 981i (B2), 816i (A2)
Zn(II)- -2579.348841 [-2579.226710] 11.1 [10.8], 71i (A1") 9.7 [10.0], 58i (A2)
Ga(III) -2724.79136916 [-2724.659359] 21.6 [20.6], 99i (A1") 19.4 [19.3], 85i (A2)
Ge(IV)+ -2876.65793452 [-2876.520686] 32.6 [32.2], 123.2 i (A1") 30.1 [29.7], 109.3 i (A2)

a Hartree, [Free energy corrected for zero point energies and entropy]. bBasis set: cc-pV5Z(5d,7f) on the metal center13, 6-31G(d) on the ligands. c Relative to the D3 geometry, kcal mol-1, [Relative free energy at 298K], d ligand out-of-plane bending mode. e Relative energy of 5-coordinate intermediate 39.4 [34.5] (cc-pV4Z basis on metal).